Recent Advances in MagnetoOptics Katsuaki Sato Department of

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Recent Advances in Magneto-Optics Katsuaki Sato Department of Applied Physics Tokyo University of Agriculture

Recent Advances in Magneto-Optics Katsuaki Sato Department of Applied Physics Tokyo University of Agriculture & Technology ICFM 2001 Crimia October 1 -5, 2001

CONTENTS 1. 2. 3. Introduction Fundamentals of Magneto-Optics Magneto-Optical Spectra • 4. Recent Advances

CONTENTS 1. 2. 3. Introduction Fundamentals of Magneto-Optics Magneto-Optical Spectra • 4. Recent Advances in Magneto-Optics • • • 5. Magneto-optics in nano-structures Nonlinear magneto-optical effect Scanning near-field magneto-optical microscope Current Status in Magneto-Optical Devices • • • 6. Experiments and theory Magneto-optical disk storages Magneto-optical isolators for optical communication Other applications Summary ICFM 2001 Crimia October 1 -5, 2001

1. Introduction • Magneto-Optical Effect:Discovered by Faraday on 1845 • Phenomenon:Change of Linear Polarization

1. Introduction • Magneto-Optical Effect:Discovered by Faraday on 1845 • Phenomenon:Change of Linear Polarization to Elliptically Polarized Light Accompanied by Rotation of Principal Axis • Cause:Difference of Optical Response between LCP and RCP • Application: – – Magneto-Optical Disk Optical Isolator Current Sensors Observation Technique ICFM 2001 Crimia October 1 -5, 2001

2. Fundamentals of Magneto-Optics • MO Effect in Wide Meaning Any change of optical

2. Fundamentals of Magneto-Optics • MO Effect in Wide Meaning Any change of optical response induced by magnetization • MO Effect in Narrow Meaning Change of intensity or polarization induced by magentization – Faraday effect – MOKE(Magneto-optical Kerr effect) – Cotton-Mouton effect ICFM 2001 Crimia October 1 -5, 2001

2. 1 Faraday Effect • (a) Faraday Configuration: – Magnetization // Light Vector •

2. 1 Faraday Effect • (a) Faraday Configuration: – Magnetization // Light Vector • (b)Voigt Configuration: – Magnetization Light Vector ICFM 2001 Crimia October 1 -5, 2001

Faraday Effect • MO effect for optical transmission – Magnetic rotation(Faraday rotation) F –

Faraday Effect • MO effect for optical transmission – Magnetic rotation(Faraday rotation) F – Magnetic Circular Dichroism(Faraday Ellipticity) F • Comparison to Natural Optical Rotation – Faraday Effect is Nonreciprocal (Double rotation for round trip) – Natural rotation is Reciprocal (Zero for round trip) • Verdet Constant – F=Vl. H (For paramagnetic and diamagnetic materials) ICFM 2001 Crimia October 1 -5, 2001

Illustration of Faraday Effect Rotation of Principal axis For linearly polarized light incidence, Elliptically

Illustration of Faraday Effect Rotation of Principal axis For linearly polarized light incidence, Elliptically Polarized light Linearly polarized light •  Elliptically polarized light goes out (MCD) • With the principal axis rotated (Magnetic rotation) ICFM 2001 Crimia October 1 -5, 2001

Faraday rotation of magnetic materials Materials Fe rotation (deg) 3. 825・ 105  figure of

Faraday rotation of magnetic materials Materials Fe rotation (deg) 3. 825・ 105  figure of merit(deg/d. B) wavelength (nm) 578 Co 1. 88・ 105 Ni 1. 3・ 105 Y 3 Fe 5 O 12 temperature (K) RT Mag. field (T) 2. 4 546 〃 2 826 120 K 0. 27 250 1150 100 K Gd 2 Bi. Fe 5 O 12 1. 01・ 104 44 800 RT Mn. Sb 2. 8・ 105 500 〃 Mn. Bi 5. 0・ 105 1. 43 633 〃 YFe. O 3 4. 9・ 103 633 〃 Nd. Fe. O 3 4. 72・ 104 633 〃 Cr. Br 3 1. 3・ 105 500 1. 5 K Eu. O 5・ 105 104 660 4. 2 K 2. 08 Cd. Cr 2 S 4 3. 8・ 103 35(80 K) 1000 4 K 0. 6 ICFM 2001 Crimia October 1 -5, 2001

2. 2 Magneto-Optical Kerr Effect • Three kinds of MO Kerr effects – Polar

2. 2 Magneto-Optical Kerr Effect • Three kinds of MO Kerr effects – Polar Kerr(Magnetization is oriented perpendicular to the suraface) – Longitudinal Kerr(Magnetization is in plane and is parallel to the plane of incidence) – Transverse Kerr (Magnetization is in plane and is perpendicular to the plane of incidence) ICFM 2001 Crimia October 1 -5, 2001

Magneto-optical Kerr effect M M M Polar Longitudinal Transverse ICFM 2001 Crimia October 1

Magneto-optical Kerr effect M M M Polar Longitudinal Transverse ICFM 2001 Crimia October 1 -5, 2001

MO Kerr rotation of magnetic materials Materials rotation Photon energy temperature field (deg) (e.

MO Kerr rotation of magnetic materials Materials rotation Photon energy temperature field (deg) (e. V) (K) (T) Fe 0. 87 0. 75 RT Co 0. 85 0. 62 〃 Ni 0. 19 3. 1 〃 Gd 0. 16 4. 3 〃 Fe 3 O 4 0. 32 1 〃 Mn. Bi 0. 7 1. 9 〃 Pt. Mn. Sb 2. 0 1. 75 1. 7 Co. S 2 1. 1 0. 8 〃 4. 2 Cr. Br 3 3. 5 2. 9 4. 2 Eu. O 6 2. 1 12 USb 0. 8 Te 9. 0 0. 8 10 4. 0 0. 2 Co. Cr 2 S 4 4. 5 0. 7 80 a-Gd. Co * 0. 3 1. 9 RT Ce. Sb 90 2 ICFM 2001 Crimia October 1 -5, 2001 0. 4

2. 3 Electromagnetism and Magnetooptics • Light is the electromagnetic wave. • Transmission of

2. 3 Electromagnetism and Magnetooptics • Light is the electromagnetic wave. • Transmission of EM wave:Maxwell equation • Medium is regareded as continuum→dielectric permeability tensor – Effect of Magnetic field→mainly to off-diagonal element • Eigenequation • →Complex refractive index:two eigenvalues eigenfunctions:right and left circularpolarization – Phase difference between RCP and LCP→rotation – Amplitude difference →circular dichroism ICFM 2001 Crimia October 1 -5, 2001

Dielectric tensor Isotromic media;M//z Invariant C 4 for 90°rotation around z-axis ICFM 2001 Crimia

Dielectric tensor Isotromic media;M//z Invariant C 4 for 90°rotation around z-axis ICFM 2001 Crimia October 1 -5, 2001

MO Equations (1) Maxwell Equation Eigenequation Eigenvalue Eigenfunction:LCP and RCP Without off-diagonal terms:No difference

MO Equations (1) Maxwell Equation Eigenequation Eigenvalue Eigenfunction:LCP and RCP Without off-diagonal terms:No difference between LCP & RCP No magnetooptical effect ICFM 2001 Crimia October 1 -5, 2001

MO Equations (2) Both diagonal and off-diagonal terms contribute to Magneto-optical effect ICFM 2001

MO Equations (2) Both diagonal and off-diagonal terms contribute to Magneto-optical effect ICFM 2001 Crimia October 1 -5, 2001

Phenomenology of MO effect Linearly polarized light can be decomposed to LCP and RCP

Phenomenology of MO effect Linearly polarized light can be decomposed to LCP and RCP Difference in phase causes rotation of the direction of Linear polarization Difference in amplitudes makes Elliptically polarized light In general, elliptically polarized light With the principal axis rotated ICFM 2001 Crimia October 1 -5, 2001

2. 4 Electronic theory of Magneto. Optics • Magnetization→Splitting of spin-states – No direct

2. 4 Electronic theory of Magneto. Optics • Magnetization→Splitting of spin-states – No direct cause of difference of optical response between LCP and RCP • Spin-orbit interaction→Splitting of orbital states – Absorption of circular polarization→Induction of circular motion of electrons • Condition for large magneto-optical response – Presence of strong (allowed) transitions – Involving elements with large spin-orbit interaction – Not directly related with Magnetization ICFM 2001 Crimia October 1 -5, 2001

Dielectric functions derived from Kubo formula where ICFM 2001 Crimia October 1 -5, 2001

Dielectric functions derived from Kubo formula where ICFM 2001 Crimia October 1 -5, 2001

Microscopic concepts of electronic polarization Wavefunction perturbed by electric field E + + -

Microscopic concepts of electronic polarization Wavefunction perturbed by electric field E + + - Unperturbed wavefunction + - = + + S-like + ・・ P-like Expansion by unperturbed orbitals ICFM 2001 Crimia October 1 -5, 2001

Orbital angular momentum-selection rules and circular dichroism px-orbital py-orbital Lz=+1 p+=px+ipy Lz=-1 p-=px-ipy Lz=0

Orbital angular momentum-selection rules and circular dichroism px-orbital py-orbital Lz=+1 p+=px+ipy Lz=-1 p-=px-ipy Lz=0 ICFM 2001 Crimia October 1 -5, 2001 s-like

Role of Spin-Orbit Interaction Jz=-3/2 Jz=-1/2 L=1 LZ=+1, 0, -1 L=0 Without magnetization LZ=0

Role of Spin-Orbit Interaction Jz=-3/2 Jz=-1/2 L=1 LZ=+1, 0, -1 L=0 Without magnetization LZ=0 Exchange splitting ICFM 2001 Crimia October 1 -5, 2001 Jz=+1/2 Jz=+3/2 Jz=-1/2 Jz=+1/2 Exchange +spin-orbit

MO lineshapes (1) 1. Diamagnetic lineshape Excited state ”xy ’xy Lz=-1 0 Lz=+1 1

MO lineshapes (1) 1. Diamagnetic lineshape Excited state ”xy ’xy Lz=-1 0 Lz=+1 1 2 1+2 Ground state Lz=0 Without magnetization With magnetization Photon energy ICFM 2001 Crimia October 1 -5, 2001 Photon energy

MO lineshapes (2) 2. Paramagnetic lineshape excited state 0 f+ f- dielectric constant f=f+

MO lineshapes (2) 2. Paramagnetic lineshape excited state 0 f+ f- dielectric constant f=f+ - f ’xy ”xy ground state without magnetic field with magnetic field photon energy (b) (a) ICFM 2001 Crimia October 1 -5, 2001

3. Magneto-Optical Spectra • • Measurement technique Magnetic garnets Metallic ferromagnet:Fe, Co, Ni Intermetallic

3. Magneto-Optical Spectra • • Measurement technique Magnetic garnets Metallic ferromagnet:Fe, Co, Ni Intermetallic compounds and alloys:Pt. Mn. Sb etc. Magnetic semiconductor:Cd. Mn. Te etc. Superlattices:Pt/Co, Fe/Au etc. Amorphous:Tb. Fe. Co, Gd. Fe. Co etc. ICFM 2001 Crimia October 1 -5, 2001

Measurement of magneto-optical spectra using retardation modulation technique i Light source monochro mator filter

Measurement of magneto-optical spectra using retardation modulation technique i Light source monochro mator filter B chopper ellipsoidal mirror polarizer j eletromagnet sample analyzer detector computer /4 P D PEM quartz Piezo e cryst lectric al A Isotropic medium fused silica Ca. F 2 Ge etc. Retardation =(2 / ) nl sin pt = 0 sin pt amp litud l e pos it ion ICFM 2001 Crimia October 1 -5, 2001

Magnetic garnets • One of the most intensively investigated magnetooptical materials • Three different

Magnetic garnets • One of the most intensively investigated magnetooptical materials • Three different cation sites; octahedral, tetrahedral and dodecahedral sites • Ferrimagnetic • Large magneto-optical effect due to strong charge -transfer transition • Enhancement of magneto-optical effect by Bisubstitution at the dodecahedral site ICFM 2001 Crimia October 1 -5, 2001

Electronic level diagram of Fe 3+ in magnetic garnets Jz= J=7/2 6 P (

Electronic level diagram of Fe 3+ in magnetic garnets Jz= J=7/2 6 P ( 6 T 6 2, T 1 g) 5 /2 - 3/2 7/2 -3/2 -7/2 3/2 -3/2 J=5/2 -3 /2 J=3/2 P+ P+ P- P- 6 S (6 A , 6 A ) 1 1 g without perturbation spin-orbit interaction -5/2 tetrahedral crystal field (Td) ICFM 2001 Crimia October 1 -5, 2001 octahedral crystal field (Oh)

Experimental and calculated magneto-optical spectra of Y 3 Fe 5 O 12 Faraday rotation

Experimental and calculated magneto-optical spectra of Y 3 Fe 5 O 12 Faraday rotation (arb. unit) 0. 8 experiment +2 0 0. 4 -2 calculation 0 -0. 4 300 400 500 Wavelength (nm) ICFM 2001 Crimia October 1 -5, 2001 600 Faraday rotation (deg/cm) x 104

Electronic states and optical transitions of Co 2+ and Co 3+ in Y 3

Electronic states and optical transitions of Co 2+ and Co 3+ in Y 3 Fe 5 O 12 (a) (b) ICFM 2001 Crimia October 1 -5, 2001

Theoretical and experimental magnetooptical spectra of Co-doped Y 3 Fe 5 O 12 ICFM

Theoretical and experimental magnetooptical spectra of Co-doped Y 3 Fe 5 O 12 ICFM 2001 Crimia October 1 -5, 2001

Theoretical and experimental MO spectra of bcc Fe Krinchik Katayama theory ICFM 2001 Crimia

Theoretical and experimental MO spectra of bcc Fe Krinchik Katayama theory ICFM 2001 Crimia October 1 -5, 2001

MO spectra of Pt. Mn. Sb Magneto-optical Kerr rotation θK and ellipticity ηK (a)

MO spectra of Pt. Mn. Sb Magneto-optical Kerr rotation θK and ellipticity ηK (a) Diagonal dielectric functions (b) ICFM 2001 Crimia October 1 -5, 2001 Off-diagonal Dielectric function (c)

Comparison of theoretical and experimental spectra of half-metallic Pt. Mn. Sb (a) (b) (c)

Comparison of theoretical and experimental spectra of half-metallic Pt. Mn. Sb (a) (b) (c) After Oppeneer (d) ICFM 2001 Crimia October 1 -5, 2001

Faraday rotation spectra (deg) Magneto-optical spectra of Cd. Mn. Te Photon Energy (e. V)

Faraday rotation spectra (deg) Magneto-optical spectra of Cd. Mn. Te Photon Energy (e. V) ICFM 2001 Crimia October 1 -5, 2001

Pt/Co superlattices Pt(10)/Co(5) Pt(18)/Co(5) simulation experiment Pt(40)/Co(20) Photon energy (e. V) Kerr rotation and

Pt/Co superlattices Pt(10)/Co(5) Pt(18)/Co(5) simulation experiment Pt(40)/Co(20) Photon energy (e. V) Kerr rotation and ellipticity(min) Pt. Co alloy rotation elliptoicity Photon energy (e. V) ICFM 2001 Crimia October 1 -5, 2001

MO spectra in RE-TM (1) Polar Kerr rotation (min) Wavelength (nm) ICFM 2001 Crimia

MO spectra in RE-TM (1) Polar Kerr rotation (min) Wavelength (nm) ICFM 2001 Crimia October 1 -5, 2001

MO spectra in R-Co Wavelength (nm) 300 Polar Kerr rotation (deg) 0 400 500

MO spectra in R-Co Wavelength (nm) 300 Polar Kerr rotation (deg) 0 400 500 600 700 -0. 2 -0. 4 -0. 6 5 4 3 Photon Energy (e. V) ICFM 2001 Crimia October 1 -5, 2001 2

MO spectra of Fe/Au superlattice ICFM 2001 Crimia October 1 -5, 2001

MO spectra of Fe/Au superlattice ICFM 2001 Crimia October 1 -5, 2001

Calculated MO spectra of Fe/Au superlattice By M. Yamaguchi et al. ICFM 2001 Crimia

Calculated MO spectra of Fe/Au superlattice By M. Yamaguchi et al. ICFM 2001 Crimia October 1 -5, 2001

Au/Fe/Au sandwich structure By Y. Suzuki et al. ICFM 2001 Crimia October 1 -5,

Au/Fe/Au sandwich structure By Y. Suzuki et al. ICFM 2001 Crimia October 1 -5, 2001

4. Recent Advances in Magneto-Optics • Nonlinear magneto-optics • Scanning near-field magneto-optical microscope (MO-SNOM)

4. Recent Advances in Magneto-Optics • Nonlinear magneto-optics • Scanning near-field magneto-optical microscope (MO-SNOM) • X-ray magneto-optical Imaging ICFM 2001 Crimia October 1 -5, 2001

NOMOKE (Nonlinear magneto-optical Kerr effect) • Why SHG is sensitive to surfaces? • Large

NOMOKE (Nonlinear magneto-optical Kerr effect) • Why SHG is sensitive to surfaces? • Large nonlinear magneto-optical effect • Experimental results on Fe/Au superlattice • Theoretical analysis • Future perspective ICFM 2001 Crimia October 1 -5, 2001

MSHG Measurement System LD pump SHG laser Electromagnet =810 nm Pulse=150 fs =532 nm

MSHG Measurement System LD pump SHG laser Electromagnet =810 nm Pulse=150 fs =532 nm Ti: sapphire P=600 m. W Mirror rep 80 MHz laser Filter Stage  controller Berek compensator Mirror Sample Analyzer Lens Filter PMT lens Chopper polarizer Photon counting Photon counter Computer ICFM 2001 Crimia October 1 -5, 2001

Sample 試料回転 Sample stage Pole p ie Rotating analyzer Filter 2 w (405 nm)

Sample 試料回転 Sample stage Pole p ie Rotating analyzer Filter 2 w (405 nm) w (810 nm) P-po larize d or S polar ized 45° light ce w (810 nm) Analyzer Optical arrangements ICFM 2001 Crimia October 1 -5, 2001

Azimuthal dependence of ・ Linear optical response ( =810 nm)    The isotropic response for the azimuthal

Azimuthal dependence of ・ Linear optical response ( =810 nm)    The isotropic response for the azimuthal angle ・ Nonlinear optical response ( =405 nm)    The 4 -fold symmetry pattern    Azimuthal pattern show 45 -rotation by reversing the magnetic field G H S SHG intensity (counts/10 sec. ) li (a) Linear (810 nm) 45 SHG intensity (counts/10 sec. ) M r a e n (b) SHG (405 nm) [Fe(3. 75 ML)/Au(3. 75 ML)] 超格子の (P in Pout)配置の線形および非線形の方位角依存性 ICFM 2001 Crimia October 1 -5, 2001

Calculated and experimental patterns : x=3. 5 SHG intensity (counts/10 sec. ) (a) Pin-Pout

Calculated and experimental patterns : x=3. 5 SHG intensity (counts/10 sec. ) (a) Pin-Pout 103 (b) Pin-Sout Dots:exp. Solid curve:calc. 103 APP=1310, B=26, C=-88 APS=-300, B=26, C=-88 (c) Sin-Pout (d) Sin-Sout 103 ASP=460, B=26, C=-88 ASS=100, B=26, C=-88 ICFM 2001 Crimia October 1 -5, 2001

Nonlinear Kerr Effect Electromagnet f = 31. 1° S-polarized light ω(810 nm) Rotating Analyzer

Nonlinear Kerr Effect Electromagnet f = 31. 1° S-polarized light ω(810 nm) Rotating Analyzer 45° Analyzer Filter 2 (405 nm) The curves show a shift for two opposite directions of magnetic field Fe(1. 75 ML)/Au(1. 75 ML) Sin ICFM 2001 Crimia October 1 -5, 2001

Nonlinear Magneto-optical Microscope P Objective lens L Sample F 1 F 2 A CCD

Nonlinear Magneto-optical Microscope P Objective lens L Sample F 1 F 2 A CCD Schematic diagram 50 m Linear and nonlinear magneto-optical images of domains in Co. Ni film ICFM 2001 Crimia October 1 -5, 2001

MO-SNOM (Scanning near-field magneto-optical microscope) • • • Near-field optics Optical fiber probe Optical

MO-SNOM (Scanning near-field magneto-optical microscope) • • • Near-field optics Optical fiber probe Optical retardation modulation technique Stokes parameter of fiber probe Observation of recorded bits on MO disk ICFM 2001 Crimia October 1 -5, 2001

Near-field Propagating wave Medium 1 Evanescent wave d i c Medium 2 i c

Near-field Propagating wave Medium 1 Evanescent wave d i c Medium 2 i c Critical angle c Total reflection and near field Evanescent field Scattered wave by a small sphere placed in the evanescent field produced by another sphere ICFM 2001 Crimia October 1 -5, 2001

Levitation control methods Quartz oscillator Fiber probe Ph oto di od LD e bimorph

Levitation control methods Quartz oscillator Fiber probe Ph oto di od LD e bimorph Sample surface Piezoelectricallydriven xyz-stage Shear force type Piezoelectricallydriven  xyz-stage Canti-lever type ICFM 2001 Crimia October 1 -5, 2001

 Collection mode(a) and illumination mode(b) ICFM 2001 Crimia October 1 -5, 2001

Collection mode(a) and illumination mode(b) ICFM 2001 Crimia October 1 -5, 2001

SNOM/AFM System Photodiode LD Compensator Polarizer Bimorph Sample PEM Optical fiber probe Filter Lock-in

SNOM/AFM System Photodiode LD Compensator Polarizer Bimorph Sample PEM Optical fiber probe Filter Lock-in Amplifier XYZ Bent fiber probe Analyzer Ar ion laser Signal generator Photomultiplier scanner Controller (SPI 3800) MO-SNOM system using PEM ICFM 2001 Crimia October 1 -5, 2001 Computer

Recorded marks on MO disk observed by MO-SNOM topography MO image ICFM 2001 Crimia

Recorded marks on MO disk observed by MO-SNOM topography MO image ICFM 2001 Crimia October 1 -5, 2001

MO-SNOM image of 0. 2 m recorded marks on Pt/Co MO disk Resolution ↓

MO-SNOM image of 0. 2 m recorded marks on Pt/Co MO disk Resolution ↓ Topographic image MO image ICFM 2001 Crimia October 1 -5, 2001 Line profile

Reflection type SNOM P. Fumagalli, A. Rosenberger, G. Eggers, A. Münnemann, N. Held, G.

Reflection type SNOM P. Fumagalli, A. Rosenberger, G. Eggers, A. Münnemann, N. Held, G. Güntherodt: Appl. Phys. Lett. 72, 2803 (1998) ICFM 2001 Crimia October 1 -5, 2001

XMCD (X-ray magnetic circular dichroism) Occupation of minority 3 d band (b) (a) md

XMCD (X-ray magnetic circular dichroism) Occupation of minority 3 d band (b) (a) md +2 +1 (6) 0 (1) (2) mj +3/2 +1/2 mj +1/2 -2 3 d (a) (3) (14) (6) (12) -1 (6) (3) -1/2 -3/2 -1/2 (b) Simulated XMCD spectra corresponding to transitions (a) and (b) in the left diagram 2 p 3/2 2 p 1/2 ICFM 2001 Crimia October 1 -5, 2001

Magnetic circular dichroism of L-edge (b) ICFM 2001 Crimia October 1 -5, 2001

Magnetic circular dichroism of L-edge (b) ICFM 2001 Crimia October 1 -5, 2001

Domain image of MO media observed using XMCD of Fe L 3 -edge Si.

Domain image of MO media observed using XMCD of Fe L 3 -edge Si. N(70 nm)/ Tb. Fe. Co(50 nm)/Si. N(20 nm)/ Al(30 nm)/Si. N(20 nm) MO 媒体 N. Takagi, H. Ishida, A. Yamaguchi, H. Noguchi, M. Kume, S. Tsunashima, M. Kumazawa, and P. Fischer: Digest Joint MORIS/APDSC 2000, Nagoya, October 30 -November 2, 2000, We. G-05, p. 114. ICFM 2001 Crimia October 1 -5, 2001

Spin dynamics in nanoscale region Ga. As high speed optical switch Th. Gerrits, H.

Spin dynamics in nanoscale region Ga. As high speed optical switch Th. Gerrits, H. van den Berg, O. Gielkens, K. J. Veenstra and Th. Rasing: Digest Joint MORIS/APDSC 2000, Nagoya, October 30 ICFM 2001 Crimia October 1 -5, 2001 November 2, 2000, Tu. C-05, p. 24.

Further Prospects -For wider range of researches- • Time (t):Ultra-short pulse→Spectroscopy using ps, fslasers,

Further Prospects -For wider range of researches- • Time (t):Ultra-short pulse→Spectroscopy using ps, fslasers, Pump-probe technique • Frequency ( ):Broad band width, Synchrotron radiation • Wavevector (k):Diffraction, scattering, magneto-optical diffraction • Length (x):Observation of nanoscale magetism, Appertureless SNOM, Spin-polarized STM, Xray microscope • Phase ( ):Sagnac interferrometer ICFM 2001 Crimia October 1 -5, 2001

5. Magneto-optical Application • Magneto-optical disk for high density storage • Optical isolators for

5. Magneto-optical Application • Magneto-optical disk for high density storage • Optical isolators for optical communication • Other applications ICFM 2001 Crimia October 1 -5, 2001

Magneto-optical (MO) Recording • Recording: Thermomagnetic recording – Magnetic recording using laser irradiation •

Magneto-optical (MO) Recording • Recording: Thermomagnetic recording – Magnetic recording using laser irradiation • Reading out: Magneto-optical effect – Magnetically induced polarization state • • MO disk, MD(Minidisk) High rewritability:more than 107 times Complex polarization optics New magnetic concepts: MSR, MAMMOS ICFM 2001 Crimia October 1 -5, 2001

History of MO recording • • • • 1962 Conger, Tomlinson Proposal for MO

History of MO recording • • • • 1962 Conger, Tomlinson Proposal for MO memory 1967 Mee Fan Proposal of beam-addressable MO recording 1971 Argard (Honeywel) MO disk using Mn. Bi films 1972 Suits(IBM) MO disk using Eu. O films 1973 Chaudhari(IBM) Compensation point recording to a-Gd. Co film 1976 Sakurai(Osaka U)Curie point recording on a-Tb. Fe films 1980 Imamura(KDD) Code-file MO memory using a-Tb. Fe films 1981 Togami(NHK) TV picture recording using a-Gd. Co MO disk 1988 Commercial appearance of 5”MO disk (650 MB) 1889 Commercial appearance of 3. 5 ”MO disk(128 MB) 1991 Aratani(Sony) MSR 1992 Sony MD 1997 Sanyo ASMO(5” 6 GB:L/G, MFM/MSR) standard 1998 Fujitsu GIGAMO(3. 5” 1. 3 GB) 2000 Sanyo, Maxell i. D-Photo(5 cmφ730 MB) ICFM 2001 Crimia October 1 -5, 2001

Structure of MO disk media • MO disk structure Al reflection layer Groove Land

Structure of MO disk media • MO disk structure Al reflection layer Groove Land Polycarbonate substrate Si. Nx layer for protection and MO-enhancement MO-recording layer (amorphous Tb. Fe. Co) Resin ICFM 2001 Crimia October 1 -5, 2001

MO recording How to record(1) • Temperature increase by focused laser beam • Magnetization

MO recording How to record(1) • Temperature increase by focused laser beam • Magnetization is reduced when T exceeds Tc • Record bits by external field when cooling M Tc Temp Tc Coil External field MO media ICFM 2001 Crimia October 1 -5, 2001 Laser spot

MO recording How to record(2) • Use of compensation point Hc writing • Amorphous

MO recording How to record(2) • Use of compensation point Hc writing • Amorphous Tb. Fe. Co: Ferrimagnet with Tcomp M • HC takes maximum at Tcomp – Stability of small recorded marks Fe, Co Tb Fe. Co Mtotal Tb RT ICFM 2001 Crimia October 1 -5, 2001 Tcomp Tc T

アモルファスTb. Fe. Co薄膜 TM R (Fe, Co) (Tb) TM (Fe, Co) R (Tb) ICFM

アモルファスTb. Fe. Co薄膜 TM R (Fe, Co) (Tb) TM (Fe, Co) R (Tb) ICFM 2001 Crimia October 1 -5, 2001

Two recording modes • Light intensity modulation (LIM): present MO – Laser light is

Two recording modes • Light intensity modulation (LIM): present MO – Laser light is modulated by electrical signal – Constant magnetic field – Elliptical marks • Magnetic field modulation (MFM):MD, ASMO – Field modulation by electrical signal – Constant laser intensity – Crescent-shaped marks Constant laser beam Modulated laser beam Constant field Modulated field (a) LIM (b) MFM ICFM 2001 Crimia October 1 -5, 2001 Magnetic head

Shape of Recorded Marks (a) LIM (b) MFM ICFM 2001 Crimia October 1 -5,

Shape of Recorded Marks (a) LIM (b) MFM ICFM 2001 Crimia October 1 -5, 2001

MO recording How to read • Magneto-optical conversion of magnetic signal to electric signal

MO recording How to read • Magneto-optical conversion of magnetic signal to electric signal D 1 LD + D 2 N S N S Differential detection Polarized Beam Splitter ICFM 2001 Crimia October 1 -5, 2001

Structure of MO Head Bias field coil Recorded marks Track pitch Focusing lens MO

Structure of MO Head Bias field coil Recorded marks Track pitch Focusing lens MO film Rotation of polarization Beam splitter mirror lens PBS (polarizing beam splitter) Laser diode Half wave-plate Photo-detector ICFM 2001 Crimia October 1 -5, 2001

Advances in MO recording 1. Super resolution 1. MSR 2. MAMMOS/DWDD 2. Use of

Advances in MO recording 1. Super resolution 1. MSR 2. MAMMOS/DWDD 2. Use of Blue Lasers 3. Near field 1. SIL 2. Super-RENS (Ag. Ox) ICFM 2001 Crimia October 1 -5, 2001

MSR (Magnetically induced super-resolution) • Resolution is determined by diffraction limit – d=0. 6λ/NA,

MSR (Magnetically induced super-resolution) • Resolution is determined by diffraction limit – d=0. 6λ/NA, where NA=n sin α – Marks smaller than wavelength cannot α be resolved d • Separation of recording and reading layers • Light intensity distribution is utilized – Magnetization is transferred only at the heated region ICFM 2001 Crimia October 1 -5, 2001

Illustration of 3 kinds of MSR ICFM 2001 Crimia October 1 -5, 2001

Illustration of 3 kinds of MSR ICFM 2001 Crimia October 1 -5, 2001

AS-MO standard ICFM 2001 Crimia October 1 -5, 2001

AS-MO standard ICFM 2001 Crimia October 1 -5, 2001

i. D-Photo specification ICFM 2001 Crimia October 1 -5, 2001

i. D-Photo specification ICFM 2001 Crimia October 1 -5, 2001

MAMMOS (magnetic amplification MO system) ICFM 2001 Crimia October 1 -5, 2001

MAMMOS (magnetic amplification MO system) ICFM 2001 Crimia October 1 -5, 2001

Super-RENS super-resolution near-field system • Ag. Ox film:decomposition and precipitation of Ag – Scattering

Super-RENS super-resolution near-field system • Ag. Ox film:decomposition and precipitation of Ag – Scattering center→near field – Ag plasmon→enhancement – reversible • Applicable to both phasechange and MO recording 高温スポット 近接場散乱 ICFM 2001 Crimia October 1 -5, 2001

To shorter wavelengths • DVD-ROM: Using 405 nm laser, successful play back of marks

To shorter wavelengths • DVD-ROM: Using 405 nm laser, successful play back of marks was attained with track pitch =0. 26 m、mark length =213 m (capacity 25 GB) using NA=0. 85 lens [i]。 [i] M. Katsumura, et al. : Digest ISOM 2000, Sept. 5 -9, 2000, Chitose, p. 18. • DVD-RW: Using 405 nm laser, read / write of recorded marks of track pitch=0. 34 m and mark length=0. 29 m in 35 m two-layered disk(capacity: 27 GB) was succeeded using NA=0. 65 lens, achieving 33 Mbps transfer rate [ii] 。 [ii] T. Akiyama, M. Uno, H. Kitaura, K. Narumi, K. Nishiuchi and N. Yamada: Digest ISOM 2000, Sept. 5 -9, 2000, Chitose, p. 116. ICFM 2001 Crimia October 1 -5, 2001

Read/Write using Blue-violet LD and SIL (solid immersion lens) NA=1. 5 405 nm 80

Read/Write using Blue-violet LD and SIL (solid immersion lens) NA=1. 5 405 nm 80 nm mark 40 GB SILhead 405 nm LD I. Ichimura et. al. (Sony), ISOM 2000 Fr. M 01 ICFM 2001 Crimia October 1 -5, 2001

SIL (solid immersion lens) ICFM 2001 Crimia October 1 -5, 2001

SIL (solid immersion lens) ICFM 2001 Crimia October 1 -5, 2001

Optical recording using SIL ICFM 2001 Crimia October 1 -5, 2001

Optical recording using SIL ICFM 2001 Crimia October 1 -5, 2001

Hybrid Recording 405 nm LD Recording head (SIL) Readout MR head Achieved 60 Gbit/in

Hybrid Recording 405 nm LD Recording head (SIL) Readout MR head Achieved 60 Gbit/in 2 H. Saga et al. Digest MORIS/APDSC 2000, Tu. E-05, p. 92. Tb. Fe. Co disk ICFM 2001 Crimia October 1 -5, 2001

Optical elements for fiber communication • Necessity of optical isolators • Principles of optical

Optical elements for fiber communication • Necessity of optical isolators • Principles of optical isolators • Structure of optical isolators – Polarization-independent type – Polarization-dependent type • Optical multiplexing and needs of optical isolators ICFM 2001 Crimia October 1 -5, 2001

Optical circuit elements proposed by Dillon (a) Rotator (b) Isolator (c) Circulator (e) Latching

Optical circuit elements proposed by Dillon (a) Rotator (b) Isolator (c) Circulator (e) Latching switch (d) Modulator ICFM 2001 Crimia October 1 -5, 2001

Optical isolator for Laser diode module Optical isolator for LD module Optical fiber Signal

Optical isolator for Laser diode module Optical isolator for LD module Optical fiber Signal source Laser diode module ICFM 2001 Crimia October 1 -5, 2001

Optical fiber amplifier and optical isolators EDFA output input Band pass filter mixer Pumping

Optical fiber amplifier and optical isolators EDFA output input Band pass filter mixer Pumping laser ICFM 2001 Crimia October 1 -5, 2001

Optical Circulator B A C D ICFM 2001 Crimia October 1 -5, 2001

Optical Circulator B A C D ICFM 2001 Crimia October 1 -5, 2001

Optical add-drop and circulator Fiber grating circulator ICFM 2001 Crimia October 1 -5, 2001

Optical add-drop and circulator Fiber grating circulator ICFM 2001 Crimia October 1 -5, 2001

Polarization dependent isolator analyzer mag. field reflected beam polarizer Faraday rotator input ICFM 2001

Polarization dependent isolator analyzer mag. field reflected beam polarizer Faraday rotator input ICFM 2001 Crimia October 1 -5, 2001

Polarization independent isolator Faraday rotator F ½ waveplate C Birefringent plate B 1 Birefringent

Polarization independent isolator Faraday rotator F ½ waveplate C Birefringent plate B 1 Birefringent plate B 2 Fiber 1 Fiber 2 Forward direction × Fiber 1 B 1 F C B 2 Fiber 2 × Reverse direction ICFM 2001 Crimia October 1 -5, 2001

Magneto-optical circulator Prism polarizer A Faraday rotator Reflection prism Half wave plate Port 2

Magneto-optical circulator Prism polarizer A Faraday rotator Reflection prism Half wave plate Port 2 Port 1 Port 4 Port 3 Prism polarizer B ICFM 2001 Crimia October 1 -5, 2001

Optical absorption in YIG ICFM 2001 Crimia October 1 -5, 2001

Optical absorption in YIG ICFM 2001 Crimia October 1 -5, 2001

Waveguide type isolators ICFM 2001 Crimia October 1 -5, 2001

Waveguide type isolators ICFM 2001 Crimia October 1 -5, 2001

Mach-Zehnder type isolator ICFM 2001 Crimia October 1 -5, 2001

Mach-Zehnder type isolator ICFM 2001 Crimia October 1 -5, 2001

Current-field sensor ICFM 2001 Crimia October 1 -5, 2001

Current-field sensor ICFM 2001 Crimia October 1 -5, 2001

Current sensors used by power engineers Before installation Magnetic core After installation Aerial wire

Current sensors used by power engineers Before installation Magnetic core After installation Aerial wire Hook Magneto-optical sensor head Fastening screw Fail-safe string Optical fiber ICFM 2001 Crimia October 1 -5, 2001

Field sensor using optical fibers ICFM 2001 Crimia October 1 -5, 2001

Field sensor using optical fibers ICFM 2001 Crimia October 1 -5, 2001

SUMMARY • Basic concepts of magneto-optics are described. • Macroscopic and microscopic origins of

SUMMARY • Basic concepts of magneto-optics are described. • Macroscopic and microscopic origins of magneto-optics are described. • Some of the recent development of magneto-optics are also given. • Some of the recent application are summarized. ICFM 2001 Crimia October 1 -5, 2001